邢唷>? ?fikoqs欹y 鳵就bjbj1遻遻.BB0$0$0$$T$T$T$P?P'<T$H$?j?:0/0/0/`p tihl|OQQQQQQlVQ0$鋗禯腳@鋗鋗Q0/0/?bbb鋗€ b0/?R0/Ob鋗Obb儴X "$"o0/P5嗗Ndy郓(;0Hlt騳:tPoo8t0$Й鋗鋗b鋗鋗鋗鋗鋗QQ,}6鋗鋗鋗H鋗鋗鋗鋗t鋗鋗鋗鋗鋗鋗鋗鋗鋗B, n: ub齉pe(W3z歔8^peKm歔-N剉擽(uXd 亯ub齉pe誰/fN蛓Km歔3z歔8^pe剉8^(u筫誰0購蛓筫誰鈋颯錘(u嶯x?z歔8^pe剉Km歔 萐颯錘(u嶯MTir3z歔8^pe剉Km歔09hncpencYt筫_剉N T ub齉pe誰颯R:N & & 0sQ.曂3z歔8^pe ub齉pe 5uMO鬾歔 x MTir Application of Bjerrum Function in Determination of Stability ConstantsABSTRACTBjerrum function method is a common method to determinate the stability constants. It can determinate the acid stability constants but also the complexes stability constants. According to the different processing methods of data, Bjerrum function method can be subdivided into 厖. Key wordsstability constants, bjerrum function, potential titration, acid, coordination compound 顅 U_ TOC \o "1-3" \h \z \u  HYPERLINK \l "_Toc402184259" 1 _  PAGEREF _Toc402184259 \h 1 HYPERLINK \l "_Toc402184260" 1.1 3z歔8^peKm歔剉aIN  PAGEREF _Toc402184260 \h 1 HYPERLINK \l "_Toc402184261" 1.2 3z歔8^peKm歔8^(u剉筫誰  PAGEREF _Toc402184261 \h 1 HYPERLINK \l "_Toc402184262" 1.2.1 Gorden誰  PAGEREF _Toc402184262 \h 1 HYPERLINK \l "_Toc402184263" 1.2.2 Monte Carlo誰  PAGEREF _Toc402184263 \h 1 HYPERLINK \l "_Toc402184264" 1.3 ub齉pe誰剉鶺,g俰礠  PAGEREF _Toc402184264 \h 1 HYPERLINK \l "_Toc402184265" 1.4 ,g噀@b\O剉錧\O  PAGEREF _Toc402184265 \h 1 HYPERLINK \l "_Toc402184266" 2 t簨钀R  PAGEREF _Toc402184266 \h 2 HYPERLINK \l "_Toc402184267" 2.1 ub齉pe誰剉鶺,gsQ鹼_  PAGEREF _Toc402184267 \h 2 HYPERLINK \l "_Toc402184268" 2.2 T蛓ub齉pe誰剉Km歔烻t  PAGEREF _Toc402184268 \h 2 HYPERLINK \l "_Toc402184269" 2.2.1 魐梴ub齉pe誰  PAGEREF _Toc402184269 \h 2 HYPERLINK \l "_Toc402184270" 2.2.2 R祂遙Tub齉pe誰  PAGEREF _Toc402184270 \h 2 HYPERLINK \l "_Toc402184271" 2.2.3 JStepeub齉pe誰  PAGEREF _Toc402184271 \h 2 HYPERLINK \l "_Toc402184272" 3 瀃寶钀R  PAGEREF _Toc402184272 \h 3 HYPERLINK \l "_Toc402184273" 3.1 闚hV孴諎BR  PAGEREF _Toc402184273 \h 3 HYPERLINK \l "_Toc402184274" 3.1.1 闚hV  PAGEREF _Toc402184274 \h 3 HYPERLINK \l "_Toc402184275" 3.1.2 諎BR  PAGEREF _Toc402184275 \h 3 HYPERLINK \l "_Toc402184276" 3.2 秐瞞剉M?R蔛h歔  PAGEREF _Toc402184276 \h 3 HYPERLINK \l "_Toc402184277" 3.2.1 NaOHh芉秐瞞剉M?R蔛h歔  PAGEREF _Toc402184277 \h 3 HYPERLINK \l "_Toc402184278" 3.2.2 /lS緮粂P[:_寕侭R剉M?R  PAGEREF _Toc402184278 \h 3 HYPERLINK \l "_Toc402184279" 3.3 瀃寶ek  PAGEREF _Toc402184279 \h 3 HYPERLINK \l "_Toc402184280" 4 觺済孴▼簨  PAGEREF _Toc402184280 \h 4 HYPERLINK \l "_Toc402184281" 4.1 YCQx慡O鹼剉觺済孴▼簨  PAGEREF _Toc402184281 \h 4 HYPERLINK \l "_Toc402184282" 4.1.1 魐梴誰  PAGEREF _Toc402184282 \h 4 HYPERLINK \l "_Toc402184283" 4.1.2 JStepe誰  PAGEREF _Toc402184283 \h 4 HYPERLINK \l "_Toc402184284" 4.1.3 R祂遙T誰  PAGEREF _Toc402184284 \h 5 HYPERLINK \l "_Toc402184285" 4.2 (l鶺xT軘SO鹼剉觺済孴▼簨  PAGEREF _Toc402184285 \h 5 HYPERLINK \l "_Toc402184286" 4.3 sQ嶯梴筫誰剉▼簨  PAGEREF _Toc402184286 \h 5 HYPERLINK \l "_Toc402184287" 4.4 sQ嶯vQ諲顣槝剉▼簨  PAGEREF _Toc402184287 \h 5 HYPERLINK \l "_Toc402184288" 5 觺簨孴U\g  PAGEREF _Toc402184288 \h 6 HYPERLINK \l "_Toc402184289" 5.1 觺簨  PAGEREF _Toc402184289 \h 6 HYPERLINK \l "_Toc402184290" 5.2 U\g  PAGEREF _Toc402184290 \h 6 HYPERLINK \l "_Toc402184291" 耂€噀.s  PAGEREF _Toc402184291 \h 7 HYPERLINK \l "_Toc402184292" " 瀼  PAGEREF _Toc402184292 \h 8 1 _ 1.1 3z歔8^peKm歔剉aIN3z歔8^pe/fSTir剉鶺,g'`(岾NN 3z歔8^pe剉Km歔/fSTirxvz剉N*N蛻亯筫b0惽忶[STir3z歔8^pe剉Km歔 颯錘& & 01.2 3z歔8^peKm歔8^(u剉筫誰1.2.1 Gorden誰鵞卂Kmx?f*g鍂Sm蔛*g鍂膥Rpe剉SO鹼 € (WBl銐3z歔8^peMR HQ梺塶x歔SO鹼剉膥Rpe孴T*N膥R剉R薡Sm[1]0(W薔(崒T粂P[:_N歔剉ag鯪 N & & 01.2.2 Monte Carlo誰& & 0HYPERLINK \l "ub齉pe誰蔛vQO縍"1.3 ub齉pe誰剉鶺,g俰礠MTirbx?z歔8^pe剉Km歔鰁 gS怺2-5]0ub齉pe誰/fKm歔3z歔8^pe剉8^(u剉筫誰 & & 0 & & 01.4 ,g噀@b\O剉錧\O,g噀\ub齉pe誰\O:NN*NteSO R+R(u魐梴ub齉pe誰0R祂遙Tub齉pe誰蔛JStepeub齉pe誰鵞MTir孴x?z歔8^pe剉Km歔蹚L垎Nxvz0;N亯ZP哊錘 N錧\O1 ╟黐哊魐梴ub齉pe誰0R祂遙Tub齉pe誰蔛JStepeub齉pe誰剉梴_ v^▼簨哊購郠蛓筫誰剉擽(uyr筽 & & 02 錘NaOH:N鬾歔BR (upH5uMO鬾歔誰R+RKm歔哊& & 0 3 & & 0& & 0 2 t簨钀R2.1 ub齉pe誰剉鶺,gsQ鹼_9hncM慚Obx懕x 蚐擽剉s^a坰Q鹼 颯錘梍0Rub齉pe[6]NMTirbx 剉T/}飝3z歔8^pe蔛秐瞞-N8n粂M慚OBRb"l粂P[ 剉s^a圫mKN魰剉sQ鹼 EMBED Equation.3  b  EMBED Equation.3  2.1 _2.1 -N  EMBED Equation.3 /fMTirbx 剉ub齉pejj=1,2,& ,n /fMTirbx 剉T/}飝3z歔8^pe[L]b[H+] /f秐瞞-N8n粂M慚OBRb"l粂P[ 剉s^a圫mvQ-N L剉5uw凃]eu 0\_2.1 橯\O錘 Nb__ 颯錘梍0Rub齉pe誰Km歔MTirbx 3z歔8^pe剉鶺,gsQ鹼_ EMBED Equation.3  b  EMBED Equation.3  2.2 )R(u_2.2  颯錘& & 0 & & 02.2 T蛓ub齉pe誰剉Km歔烻tHYPERLINK \l "魐梴ub齉pe誰Km歔3z歔8^pe剉烻t"2.2.1 魐梴ub齉pe誰 & & 02.2.2 R祂遙Tub齉pe誰 & & 02.2.3 JStepeub齉pe誰 & & 0 3 瀃寶钀R3.1 闚hV孴諎BR 3.1.1 闚hV798-MPThQ陙≧5uMO鬾歔闚^t隭N "l粂P[ 愰b'`YT5u乬^t隭N & & 03.1.2 諎BR"l'lS爺A.R. 粣飩孨2ux?l緮筟蠎鶺芉諎BR /lS緮A.R.  & & 03.2 秐瞞剉M?R蔛h歔3.2.1 NaOHh芉秐瞞剉M?R蔛h歔饄12.0g 鶹SONaOH髞100mL鏿og 竸彊4l秐銐 l忹y髞諎BR鰐 (u竸彊4lz蕬髞;`SO飝:N3L 卂h歔0\鶺芉粣飩孨2ux?l緮嶯105oC^110 oC豴髞R`蛻3\鰁  n嶯r^錻hV 稱tS髞)n0緗nx饄諷鶺芉粣飩孨2ux?l緮鍌r^翂h?.1 髞100mL鏿og R+R燫eQ50mL竸彊4l 秐銐 (u卂h歔剉NaOH秐瞞陙≧5uMO鬾歔 s^L垶[寶 N!k0NaOHh芉秐瞞剉h歔觺済翂h?.10h?.1 "l'lS爺秐瞞Smh歔鱏粣飩孨2ux?l緮(嵪?gNaOH秐瞞SO飝/mLNaOH秐瞞Sm/molL-1 10.11185.910.092620.10285.420.092930.11245.910.09323.2.2 /lS緮粂P[:_寕侭R剉M?R& & 03.3 瀃寶ek& & 0 4 觺済孴▼簨4.1 YCQx慡O鹼剉觺済孴▼簨4.1.1 魐梴誰 & & 04.1.2 JStepe誰A. 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R燫梘.Y烺齹N!k'`婼 g:-N齎 92214985.2[P]. 1993-04-01. }vfN淨.iir_眰xvz[M]//Ngb頷.iir褃f[蹚U\.S琋:貧I{Ye瞼鶴Hr>y 1998:146-163.煍噀裇.^椏~'`膲R(W颯胵襨irM憂-N剉擽(u[C]//u嵁s.袕y{f[剉t簨N擽(u:-N齎袕y{f[O,{擭J\'YO簨噀茤.墘[:墘[5uP[褃€b'Yf[鶴Hr>y 1996:468-471. _0u銻.j痳DNA揯Nu}T&Otf[R[N].'YO褃€b 2000-11-12(7).hQ齎酧o`N噀.sh芉S€b/g訷XTO.噀.sW刄_:,{4钀R ^梖ND崣e: GB/T 3792.4-2009[S].S琋:-N齎h芉鶴Hr>y 2010:3.'劗?鶴HrN酧o`S葟篘隷f廠怺EB/OL].(2001-12-19)[2002-04-15].http://www.creader. com/news/20011219/200112190019.html.Dublin core metadata element set: version 1.1[EB/OL].(2012-06-14)[2014-06-11].http:// dublincore.org/documents/dces/. 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